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  6. Anisotropic antiferromagnetic order in EuPd3Si2
 
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Title(s)
TitleLanguage
Anisotropic antiferromagnetic order in EuPd3Si2
en
 
Author(s)
NameORCIDGNDAffiliation
Michelle Ocker
0009-0003-4975-871X
Physics 
 
Project(s)
TRR 288: Elastic Tuning and Response of Electronic Quantum Phases of Matter 
 
Faculty
13 Physics
 
Date Issued
07 October 2025
 
Publisher(s)
Goethe-Universität Frankfurt
 
Handle
https://gude.uni-frankfurt.de/handle/gude/666
 
DOI
10.25716/gude.0k6n-7bfc
 

Type(s) of data
DataPaper
 
Language(s)
en
 
Abstract(s)
AbstractLanguage
Single crystals of EuPd$_3$Si$_2$ were grown using a high-temperature EuPd-flux method. The material was structurally and chemically characterized by single-crystal x-ray diffraction, powder x-ray diffraction, Laue method and energy-dispersive x-ray spectroscopy.
The structural analysis confirmed the orthorhombic crystal structure (space group $Imma$) but revealed differences in the lattice parameters and bond distances in comparison to previous work by Sharma et al.. \\
The composition is close to the ideal 1:3:2 stoichiometry with an occupation of 7 \% of the Si sites by Pd. The heat capacity, electrical resistivity, and magnetic susceptibility show two magnetic transitions indicating antiferromagnetic ordering below $T_{\rm N1}=$ 61\,K and a spin reorientation at $T_{\rm N2}=$ 40\,K. The orthorhombic material shows magnetic anisotropy with field applied along the three main symmetry axes, which is summarized in the temperature-field phase diagrams. The susceptibility data hint to an alignment of the magnetic moments along $[100]$ between $T_{\rm N1}$ and $T_{\rm N2}$. Below $T_{\rm N2}$ the magnetic structure changes to an arrangement with moments canted away from $[100]$. In contrast to published workby Sharma et al., the single crystals investigated in this study show AFM order below $T_{\rm N1}$ instead of ferromagnetism that sets in at higher $T_{\rm C1}=78\,\rm K$ which might originate from certain differences in the structure, composition or defects that have an impact on the dominant coupling constants of the RKKY interaction.
 

License
Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International (CC BY-NC-ND 4.0) cclicense-logocclicense-logocclicense-logocclicense-logo
 

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Oct 13, 2025
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