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  6. TR 288: Elastic Tuning and Response of Electronic Quantum Phases of Matter of Electronic Q
  7. TR 288 - Elasto-Q-Mat: Research Data
  8. Epitaxial EuPd2Si2 thin films
 
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Title(s)
TitleLanguage
Epitaxial EuPd2Si2 thin films
en
 
Author(s)
NameORCIDGNDAffiliation
Kölsch, Sebastian 
0000-0003-3596-964X
Faculty of Physics 
 
Project(s)
Strain effects in thin films of correlated intermetallic compounds (A04) 
 
Faculty
13 Physics
 
DFG-Subject
307-01 Experimental Condensed Matter Physics
 
Date Issued
November 2022
 
Publisher(s)
Goethe-Universität Frankfurt
 
Handle
https://gude.uni-frankfurt.de/handle/gude/257
 
DOI
10.25716/gude.1666-ssnt
 

Type(s) of data
Text
 
Language(s)
en
 
Subject Keyword(s)
  • EuPd2Si2 thin film

  • strain

  • MBE

  • Thin film growth

  • Europium

 
Abstract(s)
AbstractLanguage
Bulk EuPd2Si2 show a temperature-driven valence transisition of europium from ~+2 above 200 K to~+3 below 100 K, which is correlated with a shrinking by approximatly 2 % of the crystal lattice along the two a-axes. Due to this interconnection between lattice and electronic degrees of freedom the influence of strain in epitaxial thin films is particularly interesting. Ambient X-ray diffraction (XRD) confirms an epitaxial relationship of tetragonal EuPd2Si2 on MgO(001) with an out-of plane c-axis orientation for the thin film, whereby the a-axes of both lattices align. XRD at low temperatures reveals a strong coupling of the thin film lattice to the substrate, showing no abrupt compression over the temperature range from 300 to 10 K. Hard X-ray photoelectron spectroscopy at 300 and 20 K reveals a temperature-independent valence of +2.0 for Eu. The evolving biaxial tensile strain upon cooling is suggested to suppress the valence transition. Instead low temperature transport measurements of the resistivity and the Hall effect in a magnetic field up to 5 T point to a film thickness independent phase transition at 16-20 K, indicating magnetic ordering.
en
 

Funder(s)
NameType of identifierFunder identifierAward numberAward titleAward URI
DFG German Research Fundation
4222213477
TRR 288 Elastic Tuning and Response of Electronic Quantum Phases of Matter
 

License
Creative Commons Attribution 4.0 International (CC BY 4.0) cclicense-logocclicense-logo
 

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May 9, 2025
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