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Title(s)
Title | Language |
Anisotropic antiferromagnetic order in EuPd3Si2 | en |
Author(s)
Name | ORCID | GND | Affiliation |
Michelle Ocker |
Faculty
13 Physics
Date Issued
07 October 2025
Publisher(s)
Goethe-Universität Frankfurt
Type(s) of data
DataPaper
Language(s)
en
Abstract(s)
Abstract | Language |
Single crystals of EuPd$_3$Si$_2$ were grown using a high-temperature EuPd-flux method. The material was structurally and chemically characterized by single-crystal x-ray diffraction, powder x-ray diffraction, Laue method and energy-dispersive x-ray spectroscopy. The structural analysis confirmed the orthorhombic crystal structure (space group $Imma$) but revealed differences in the lattice parameters and bond distances in comparison to previous work by Sharma et al.. \\ The composition is close to the ideal 1:3:2 stoichiometry with an occupation of 7 \% of the Si sites by Pd. The heat capacity, electrical resistivity, and magnetic susceptibility show two magnetic transitions indicating antiferromagnetic ordering below $T_{\rm N1}=$ 61\,K and a spin reorientation at $T_{\rm N2}=$ 40\,K. The orthorhombic material shows magnetic anisotropy with field applied along the three main symmetry axes, which is summarized in the temperature-field phase diagrams. The susceptibility data hint to an alignment of the magnetic moments along $[100]$ between $T_{\rm N1}$ and $T_{\rm N2}$. Below $T_{\rm N2}$ the magnetic structure changes to an arrangement with moments canted away from $[100]$. In contrast to published workby Sharma et al., the single crystals investigated in this study show AFM order below $T_{\rm N1}$ instead of ferromagnetism that sets in at higher $T_{\rm C1}=78\,\rm K$ which might originate from certain differences in the structure, composition or defects that have an impact on the dominant coupling constants of the RKKY interaction. |
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Oct 13, 2025
Oct 13, 2025
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Acquisition Date
Oct 13, 2025
Oct 13, 2025